TiO2-Based Heterostructure Containing g-C3N4 for an Effective Photocatalytic Treatment of a Textile Dye
نویسندگان
چکیده
Water pollution has become a serious environmental issue. The textile industries using dyes are considered to be one of the most polluting all industrial sectors. application solar-light semiconductor catalysts in wastewater treatment, among which TiO2 can prospective candidate, is limited by rapid recombination photogenerated charge carriers. To address these limitations, was tailored with graphitic carbon nitride (g-C3N4) develop heterostructure g-C3N4@TiO2. Herein, simple hydrothermal synthesis TiO2@g-C3N4 presented, titanium isopropoxide (TTIP) and urea as precursors. morphological optical properties structure g-C3N4, TiO2, prepared (with different wt.% up 32%), were analyzed various laboratory methods. photocatalytic activity studied through degradation methylene blue (MB) aqueous solution under UV-A simulated solar irradiation. results showed that amount g-C3N4 irradiation source important influences on efficiency MB removal Photocatalytic also examined realistic conditions, such natural sunlight environments. synthesized g-C3N4@TiO2 nanocomposite superior comparison pure thus promising new photocatalyst for real-life implementation. mechanism investigated scavengers electrons, holes, hydroxyl radicals find responsible species degradation.
منابع مشابه
Photocatalytic application of TiO2/SiO2-based magnetic nanocomposite (Fe3O4@SiO2/TiO2) for reusing of textile wastewater
In this research we have developed a treatment method for textile wastewater by TiO2/SiO2-based magnetic nanocomposite. Textile wastewater includes a large variety of dyes and chemicals and needs treatments. This manuscript presents a facile method for removing dyes from the textile wastewater by using TiO2/SiO2-based nanocomposite (Fe3O<su...
متن کاملUV/Tio2 photocatalytic reactor for real textile wastewaters treatment.
Textile dye wastewaters are characterized by strong colour, salts and other additives, high pH, temperature, chemical oxygen demand (COD) and biodegradable materials. Being aesthetically and environmentally unacceptable, these wastewaters need to be treated before their discharge. Anaerobic bioprocesses have been proposed as being environmentally friendly and relatively cheap; however, when app...
متن کاملSimultaneous photocatalytic and microbial degradation of dye-containing wastewater by a novel g-C3N4-P25/photosynthetic bacteria composite
Azo dyes are very resistant to light-induced fading and biodegradation. Existing advanced oxidative pre-treatment methods based on the generation of non-selective radicals cannot efficiently remove these dyes from wastewater streams, and post-treatment oxidative dye removal is problematic because it may leave many byproducts with unknown toxicity profiles in the outgoing water, or cause expensi...
متن کاملPt‐Decorated g‐C3N4/TiO2 Nanotube Arrays with Enhanced Visible‐Light Photocatalytic Activity for H2 Evolution
Aligned TiO2 nanotube layers (TiNTs) grown by self-organizing anodization of a Ti-substrate in a fluoride-based electrolyte were decorated with graphitic-phase C3N4 (g-C3N4) via a facile chemical vapor deposition approach. In comparison with classical TiO2 nanotubes (anatase), the g-C3N4/TiNTs show an onset of the photocurrent at 2.4 eV (vs. 3.2 eV for anatase) with a considerably high photocur...
متن کاملCodeposition of Fe3O4 Nanoparticles Sandwiched Between g-C3N4 and TiO2 Nanosheets: Structure, Characterization and High Photocatalytic Activity for Efficiently Degradation of Dye Pollutants
Novel ternary nanocomposite photocatalysts based on g-C3N4/Fe3O4/TiO2 nanosheet were synthesized using simple solid combustion, hydrothermal and wetness impregnation methods. The g-C3N4 nanosheet (2D)/ Fe3O4/ TiO2 nanosheet (2D) triad-interface nanocomposite arranged in the form of Fe3O4 nanoparticle was sandwiched and well dispersed on the surface between g-C3N4 and TiO2 nanosheets. The synthe...
متن کاملذخیره در منابع من
با ذخیره ی این منبع در منابع من، دسترسی به آن را برای استفاده های بعدی آسان تر کنید
ژورنال
عنوان ژورنال: Catalysts
سال: 2022
ISSN: ['2073-4344']
DOI: https://doi.org/10.3390/catal12121554